“Soaking-in-water” strategy stimulated starch/poly(vinyl alcohol)-based flexible hydrogel with heterogeneous network for highly sensitive underwater wearable sensor

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  • Xueting Li
  • Rongtong He
  • Xingxun Liu
  • Andreas Blennow
  • Qichao Ye
  • Bingbing Hong
  • Xiaonan Li
  • Lu Lu
  • Bo Cui

Underwater wearable sensors utilizing conductive hydrogels have garnered significant attention in recent years. However, the response sensitivity to the mechanical strain, quantified by the gauge factor (GF), of most hydrogels is noticeably diminished when submerged in water, and little consideration has been given to the GF value of sensors operating both in air and underwater. Consequently, the development of underwater sensors with high sensitivity in aquatic environments remains a challenge. In this study, we propose a “soaking-in-water” strategy to enhance the sensitivity of the wearable sensor based on starch/poly(vinyl alcohol)/graphene oxide/ionic liquid hydrogel. Through this approach, the maximum GF of the hydrogel underwater was improved to 9.71, representing an 86.7% increase compared to the unsoaked hydrogel (GF of 5.20). Furthermore, the hydrogel demonstrated adjustable conductivity (from 0.26 to 1.82 S·m−1) and tensile properties (from 0.05 MPa at 244% to 0.21 MPa at 527%). The hydrogel underwent the processes of water-absorbing swelling, exudation of ionic liquid and water-repelling shrinkage. The enhancement in sensitivity and swelling mechanism of the hydrogel were closely linked to the movement of ions and water between the hydrogel and soaking water. Leveraging these properties, we further developed an underwater strain sensor capable of monitoring human motions underwater, offering quick, effective, and stable signal transmission. The proposed soaking method represents a promising avenue for improving the sensitivity of hydrogel sensors, providing a facile strategy for achieving accurate and efficient underwater monitoring applications.

OriginalsprogEngelsk
Artikelnummere01049
TidsskriftSustainable Materials and Technologies
Vol/bind41
Antal sider13
ISSN2214-9937
DOI
StatusUdgivet - 2024

Bibliografisk note

Funding Information:
This work was supported by Natural Science Foundation of Shandong Province (No. ZR2022MC178), Major Innovation Pilot Project of Integration of Science, Education and Industry of Qilu University of Technology (Shandong Academy of Science) (No. 2022JBZ01-08), National Training Program of Innovation and Entrepreneurship for Undergraduates (No. 202310431053), Shandong Province undergraduate teaching reform research project (No. M2023003, Z2022193), Undergraduate teaching reform research key project of Qilu University of Technology (Shandong Academy of Science) (No. 2022zd07), Graduate education teaching reform project of Qilu University of Technology (Shandong Academy of Science) (No. YJG23YB011), and Qilu University of Technology (Shandong Academy of Sciences) school-level Training Key Program of Innovation and Entrepreneurship for Undergraduates (2024-38).

Publisher Copyright:
© 2024 Elsevier B.V.

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